Process for the manufacture of chiral aldehydes

C - Chemistry – Metallurgy – 07 – D

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260/306.2, 260/3

C07D 405/04 (2006.01) C07D 307/33 (2006.01) C07D 317/20 (2006.01) C07D 317/26 (2006.01) C07D 317/28 (2006.01) C07D 405/14 (2006.01) C07D 407/04 (2006.01)

Patent

CA 1224789

Abstract The manufacture of chiral aldehydes of the general formula Image in which R3 and R4 each individually repre- sent hydrogen or lower alkyl or together represent lower alkylene, by reacting a lactone of the general formula Image II in which R3 and R4 have the significance given above, with an alkali metal metaperiodate is described. The chiral aldehydes of formula I can be used for the manufacture of chiral .beta.-lactams of the general formula Image III in which R1 represents a readily cleavable protecting group, R2 represents benzyloxy- carbonylamino, azido, phthalimido or the group R5R6C=CR7-NH-, wherein R5 repre- sents lower alkanoyl, lower alkoxycarbonyl or benzoyl, R6 represents hydrogen, lower alkyl, lower alkanoyl, lower alkoxycarbonyl or cyano and R7 represents hydrogen or lower alkyl, and R3 and R4 each individually represent hydrogen or lower alkyl or to- gether represent lower alkylene. The chiral .beta.-lactams of formula III are intermediates for the manufacture of antimicrobially active .beta.-lactams.

446804

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