Process for production of high-molecular-weight polyarylene...

C - Chemistry – Metallurgy – 08 – G

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C08G 75/02 (2006.01)

Patent

CA 1254345

ABSTRACT OF THE DISCLOSURE A process for the preparation of a high-molecular- weight polyarylene sulfide, which comprises subjecting an alkali metal sulfide such as sodium sulfide and a dihalo aromatic compound such as dichlorobenzene to dehalogenation sulfidation reaction in an organic amide solvent, wherein the reaction is carried out by using a reaction vessel in which at least the portion which the reaction liquid contacts is made of titanium, through at least the following two steps: (1) the step of carrying out the reaction at a temperature of 180 to 235°C in the presence of water in an amount of 2.4 to 10 moles per mole of the alkali metal sulfide so that the conversion of the dihalo aromatic compound is at least 50% and the melt viscosity of the formed polyarylene sulfide does not exceed 500 P, and (2) the step of elevating the temperature to 245 to 290°C in the presence of water in an amount of 2.5 to 10 moles per mole of the alkali metal sulfide by or without adding water to the reaction system and carrying out the reaction. The titanium reaction vessel is used for at least the step (1) and, preferably, for both the steps (1) and (2). The two-step reaction is advantageous in producing high molecular weight polyarylene sulfide.

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