Supported metal catalyst, preparation and applications for...

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B01J 23/38 (2006.01) B01J 23/10 (2006.01) B01J 23/40 (2006.01) B01J 35/10 (2006.01) B01J 37/02 (2006.01)

Patent

CA 2378919

The invention concerns a supported metal catalyst based on at least one metal selected in the group M consisting of palladium, platinum, ruthenium, rhodium, iridium, holmium, osmium and gold, used for directly making hydrogen peroxide from hydrogen and oxygen. The invention also concerns a method for making said catalyst comprising successively an impregnating step with a solution based on one or several salt(s) of at least one metal of group M on a support, and a reduction step characterised in that at the end of the reduction step, the catalyst is treated with an aqueous acid solution comprising bromine and bromide ions. The catalyst is characterised by metal or crystallised metal aggregates with size ranging between 0.1 and 20 microns and preferably between 0.1 and 10 microns. The supported bimetal catalyst is preferred, for example Pd-Pt, Au-Pt, Pd-Ho and Pd-Au.

La présente invention concerne un catalyseur métallique supporté à base d'au moins un métal choisi dans le groupe M formé de palladium, platine, ruthénium, rhodium, d'iridium, d'holmium, d'osmium et d'or, utilisé dans la fabrication directe du peroxyde d'hydrogène à partir d'hydrogène et d'oxygène. Le procédé de préparation du catalyseur comprenant successivement une étape d'imprégnation d'une solution à base d'un ou plusieurs sel(s) d'au moins un métal du groupe M sur un support, et une étape de réduction caractérisée en ce qu'à l'issue de l'étape de réduction, le catalyseur est soumis à un traitement avec une solution aqueuse acide comprenant du brome et des ions bromure. Le catalyseur est caractérisé par des amas de métal ou métaux cristallisés de taille comprise entre 0,1 et 20 microns et de préférence comprise entre 0,1 et 10 microns. Le catalyseur bimétallique supporté est préféré, par exemple Pd-Pt, Au-Pt, Pd-Ho et Pd-Au.

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