Production of bridged hafnocenes

C - Chemistry – Metallurgy – 07 – F

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C07F 17/00 (2006.01) C08F 10/00 (2006.01)

Patent

CA 2299536

Racemic, bridged hafnocene is produced in enhanced yield by reacting a hafnium halide-aliphatic polyether adduct that has been formed and/or heated at one or more temperatures of at least 40 ~C, and a metallated bis(cyclopentadienyl- moiety-containing) ligand, at one or more temperatures for a sufficient period of time such that a racemic, bridged hafnocene is produced. The reaction is performed in the substantial absence of tetrahydrofuran and/or any other ether solvent or diluent that causes the formation of a tarry residue in the reaction mixture.

On produit un hafnocène ponté, racémique, avec un rendement amélioré, en faisant réagir un produit d'addition d'halogénure d'hafnium-polyéther alipathique ayant été formé et/ou chauffé à une ou plusieurs températures d'au moins 40 ·C, et un ligand contenant une fraction de bis(cyclopentadiényle) métallée, à une ou plusieurs températures pendant une période de temps suffisante pour produire un hafnocène ponté, racémique. La réaction est réalisée en l'absence sensible de tétrahydrofurane et/ou de tout autre solvant ou diluant à base d'éther entraînant la formation d'un résidu goudronneux dans le mélange de réaction.

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