Process for the preparation of transition metal complexes...

C - Chemistry – Metallurgy – 07 – F

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C07F 17/00 (2006.01) C07F 17/02 (2006.01)

Patent

CA 2112919

The invention relates to a process for the preparation of transition metal complexes having monosubstituted cyclopentadienyl ligands of the general formula (see fig. I) in which monomeric cyclopentadiene is reacted with organic halides or pseudohalides, using a mixture of an alkyli metal oxide or hydroxide and an alkaline earth metal oxide ox hydroxide as metallating agent in glycol diethers as solvent, to form the intermediate monosubstituted cyclopentadiene, which in situ is metallated and reacted with a transition metal halide to give the final product.

Méthode pour préparer des complexes de métal de transition, renfermant des ligands cyclopentadiényliques avec monosubstitution de formule générale (voir fig. I), dans laquelle on fait réagir du cyclopentadiène monomère avec des halogénures ou des pseudohalogénures organiques, à l'aide d'un mélange d'un oxyde ou hydroxyde de métal alcalin et d'un oxyde ou hydroxyde de métal alcalino-terreux, comme agent de métallation dans des diéthers-oxydes de glycol comme solvants, pour l'obtention de cyclopentadiène intermédiaire avec monosubstitution, qui est soumis à une métallation in situ et à une réaction avec un halogénure de métal de transition pour former le produit final.

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