Process for producing isocyanates using diaryl carbonate

C - Chemistry – Metallurgy – 07 – C

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C07C 263/04 (2006.01) C07C 265/14 (2006.01) C07C 269/04 (2006.01) C07C 271/54 (2006.01)

Patent

CA 2721357

An object of the present invention is to provide a process that enables isocyanate to be produced stably over a long period of time and at high yield without encountering problems of the prior art during production of isocyanate without using phosgene. The present invention provides an isocyanate production process including the steps of: obtaining a reaction mixture containing an aryl carbamate having an aryl group originating in a diaryl carbonate, an aromatic hydroxy compound originating in a diaryl carbonate, and a diaryl carbonate, by reacting a diaryl carbonate and an amine compound in the presence of a reaction solvent in the form of an aromatic hydroxy compound; transferring the reaction mixture to a thermal decomposition reaction vessel; and obtaining isocyanate by applying the aryl carbamate to a thermal decomposition reaction, wherein the reaction vessel in which the reaction between the diaryl carbonate and the amine compound is carried out and the thermal decomposition reaction vessel for the aryl carbamate are different.

La présente invention concerne un procédé de production qui, en produisant un isocyanate sans utiliser de phosgène, ne présente pas les différents problèmes rencontrés dans l'art antérieur et peut stablement produire l'isocyanate en un rendement élevé pendant une longue période de temps. Le procédé de production comprend l'étape consistant à faire réagir le diaryl carbonate avec un composé amine en présence d'un composé hydroxy aromatique en tant que solvant de réaction pour donner un mélange réactionnel contenant un aryl carbamate contenant un groupe aryle dérivé d'un diaryl carbonate, un composé hydroxy aromatique dérivé d'un diaryl carbonate, et un diaryl carbonate, l'étape consistant à transférer le mélange réactionnel à un réacteur de décomposition thermique, et l'étape consistant à thermiquement décomposer l'aryl carbamate pour obtenir un isocyanate. Dans ce procédé de production, le réacteur pour la réaction du diaryl carbonate avec le composé amine est différent du réacteur de décomposition thermique de l'aryl carbamate.

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