Nitrogen-containing group 13 anionic complexes for olefin...

C - Chemistry – Metallurgy – 08 – F

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C08F 4/643 (2006.01) C08F 4/02 (2006.01) C08F 4/645 (2006.01) C08F 10/02 (2006.01) C08F 210/02 (2006.01) C08F 4/659 (2006.01) C08F 4/6592 (2006.01) C08F 210/16 (2006.01)

Patent

CA 2330882

This description addresses a process for the preparation of polyolefins from one or more olefinic monomers comprising combining said olefins under olefin polymerization conditions with an organometallic catalyst compound that is activated for olefin polymerization by reaction with a Group 13 element cocatalyst complex comprising at least one halogenated, nitrogen-containing aromatic group ligand. High number-average molecular weight polymers and copolymers at high rates of productivity were observed from the user of metallocene catalysts complexes when activated with [(C6H5)3C][(C6F5)3B(C5F4N)].

L'invention concerne un procédé de préparation de polyoléfines à partir d'un ou plusieurs monomères oléfiniques. Ledit procédé consiste à combiner lesdites oléfines dans des conditions de polymérisation d'oléfines, avec un composé catalysant organométallique activé pour la polymérisation d'oléfines, par la mise en réaction avec un complexe co-catalysant élémentaire de groupe 13 comprenant au moins un ligand du groupe aromatique contenant de l'azote, halogéné. On a constaté que l'utilisation de complexes catalyseurs métallocènes lorsqu'ils sont activés avec [(C¿6?H¿5?) C¿3?C][(C¿6?F¿5?)¿3?B(C¿5?F¿4?N)] permettait la production en grande quantité de copolymères et de polymère à poids moléculaire moyen en nombre élevé.

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