Process for halogenation of isomonoolefin/para-alkylstyrene...

C - Chemistry – Metallurgy – 08 – F

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C08F 8/20 (2006.01) C08F 8/22 (2006.01)

Patent

CA 2257820

A process for halogenating a copolymer of a C4-C7 isomonoolefin, e.g. isobutylene, and a para-alkylstyrene, e.g., para-methylstyrene, is disclosed. Increased halogenation efficiency is achieved by conduction the reaction under free radical halogenation conditions and in the presence of an oxidizing agent, e.g. hydrogen peroxide, which oxidizes hydrogen halide generated in situ in the reaction back to free halogen. The oxidizing agent is preferably not added to the reaction medium until after first stage halogenation is substantially completed.

Cette invention concerne un procédé d'halogénation d'un copolymère constitué d'une iso-mono-oléfine C¿4? à C¿7?, telle que l'isobutylène, et d'un para-alkylstyrène, tel que le para-méthylstyrène. On parvient à accroître le rendement de l'halogénation en effectuant la réaction dans des conditions d'halogénation radicalaire et en présence d'un agent d'oxydation, tel que le peroxyde d'hydrogène, qui oxyde l'halogénure d'hydrogène produit in-situ au cours de la réaction et le retransforme en halogène libre. De préférence, on n'ajoute pas ledit agent d'oxydation au milieu réactionnel avant que l'halogénation de première étape ne soit pratiquement achevée.

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