Polymerization of alpha-olefins with transition metal...

C - Chemistry – Metallurgy – 07 – F

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C07F 17/00 (2006.01) B01J 31/18 (2006.01) C07F 7/00 (2006.01) C07F 7/28 (2006.01) C08F 4/642 (2006.01) C08F 10/00 (2006.01) C08F 10/02 (2006.01) C08F 4/659 (2006.01) C08F 110/02 (2006.01) C08F 210/16 (2006.01)

Patent

CA 2218638

Disclosed is a novel bidentate pyridine transition metal catalyst having general formula (1), where Y is 0, S, NR, (2), or (3), each R is independently selected from hydrogen or C1 to C6 alkyl, each R' is independently selected from C1 to C6 alkyl, C1 to C6 alkoxy, C6 to C16 aryl, halogen, or CF3, M is titanium, zirconium, or hafnium, each X is independently selected from halogen, C1 to C6 alkyl, C1 to C6 alkoxy, or (4), L is X, cyclopentadienyl, C1 to C6 alkyl substituted cyclopentadienyl, indenyl, fluorenyl, or (5), "m" is 0 to 4, and "n" is 1 to 4. Also disclosed is a method of making a poly-.alpha.-olefin comprising polymerizing an .alpha.-olefin monomer using that catalyst or a catalyst that has general formula (6), where Y, M, L, X, and R' were previously defined and each "p" is independently selected from 0 to 3.

La présente invention décrit un nouveau catalyseur renfermant des métaux de transition à base de pyridine bidentée de formule (1), dans laquelle Y représente O, S, NR, (2) ou (3), chaque R est indépendamment choisi parmi hydrogène ou alkyle C1 à C6, chaque R' est indépendamment choisi parmi alkyle C1 à C6, alkoxy C1 à C6, aryle C6 à C16, halogène ou CF3, M représente titane, zirconium ou hafnium, chaque X est indépendamment choisi parmi halogène, alkyle C1 à C6, alkoxy C1 à C6 ou (4); L représente X, cyclopentadiényle, cyclopentadiényle substitué par alkyle C1 à C6, indényle, fluorényle ou (5); "m" est compris entre 0 et 4, et "n" est compris entre 1 et 4. L'invention décrit également un procédé de fabrication d'une poly- alpha -oléfine consistant à polymériser un monomère d' alpha -oléfine en utilisant ledit catalyseur ou un catalyseur de formule générale (6), où Y, M, L, X et R' sont tels que définis précédemment et où chaque "p" est indépendamment choisi entre 0 et 3.

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