Process for the preparation of benzylamines

C - Chemistry – Metallurgy – 07 – D

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260/247.47, 260/

C07D 295/18 (2006.01) C07D 295/185 (2006.01)

Patent

CA 1050023

ABSTRACT OF THE DISCLOSURE The invention relates to a new process for the preparation of benzylamine derivatives of the general formula Image (I) (wherein Hal represents a chlorine or bromine atom; R1 represents a hydrogen, chlorine or bromine atom; R2 represents a hydrogen atom or an alkyl group with 1 to 3 carbon atoms; and either R3 represents a cyclohexyl or hydroxy- cyclohexyl group and R4 represents a hydrogen atom or R3 represents an isopropylaminocarbonylmethyl or a morpholine-carbonylmethyl group and R4 represents a hydrogen atom or a benzyl group) and acid addition salts thereof, which process comprises reacting a compound of formula Image (II) (wherein R1, R4 and Hal are as hereinbefore defined and X represents a nucleophilic leaving group) with a compound of formula Image (III) (wherein R2 and R3 are as hereinbefore defined) and if desired subsequently converting the compound of formula I thereby obtained into an acid addition salt thereof having valuable physiological properties, in particular a secretolytic, antitussive and/or respiration stimulating activity. The new process comprises aminating a reactive derivative of the corresponding benzyl alcohol. Examples of the preparation of some benzylamine derivatives by means of the new process are given.

194467

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