2, 2-dibromo-azasteroids and their use in a method for...

C - Chemistry – Metallurgy – 07 – J

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C07J 73/00 (2006.01)

Patent

CA 2271974

A process for introducing a 1,2-double bond into 17.beta.-substituted-3-oxo-4- azasteroids includes the preparation of novel 2,2-dibromo-4-azasteroids by a three step process comprising oxalylation, reaction with excess bromine, and removal of the oxalyl group. This process is preferably carried out at temperatures at or above -20°C and results in a high yield of the 2,2-dibromo-4-azasteroid. The 2,2-dibromo-4-azasteroid can be converted to the corresponding 17.beta.-substituted-4-aza-5.alpha.-androst-1-ene-3-one by at least two processes, one of which involves correcting the oxidation state at the 2-carbon and then introducing the 1,2- double bond, and the other of which involves introducing the unsaturation to produce a vinyl bromide followed by correcting the oxidation state of the 2-carbon. Preferably, the dibromo compound is reacted with thiophenol to produce a 2-phenylthio intermediate, followed by oxidation of the phenylthio group to a sulfoxide and 1,2-elimination of the sulfoxide group to create the 1,2- double bond.

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