Acrylate-containing compositions and their polymerisation

C - Chemistry – Metallurgy – 08 – F

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402/343, 204/91.

C08F 22/10 (2006.01) C08F 20/40 (2006.01) C08K 5/37 (2006.01) C09D 4/00 (2006.01)

Patent

CA 1190699

- 1 - ABSTRACT OF THE DISCLOSURE Polymerisable compositions comprise a) a compound containing both i) at least one acryloyloxy or methacryloyloxy group, ii) at least one allyl, methallyl, or 1-propenyl group attached directly to a carbon atom which forms part of an aromatic nucleus or to an oxygen atom or an oxycarbonyl group which are in turn directly attached to such a carbon atom, the total of the said groups i) and ii) being at least three, and b) a compound containing at least two mercaptan groups directly attached to aliphatic carbon atoms, in a proportion as to supply at least 0.8 such mercaptan group per allyl, methallyl or 1-propenyl group in a) but less than 1.0 such mercaptan group in a) per acryloyl, methacryloyl, allyl, methallyl, or 1-propenyl group Examples of a) are 2,2-bis(3-allyl-4-(methacryloyloxy)phenyl)- - 2 - propane, bis(3-methallyl-4-(methacryloyloxy)phenyl)methane, 2,2-bis(3-allyl-4-(3-(methacryloyloxy)-2 hydroxypropoxy)phenyl)propane, 2,6-dimethallylphenyl acrylate, 1-(allyloxycarbonyl)-2,4- and 2,5-bis(3-(methacryloyloxy)-2-hydroxypropoxycarbonyl)benzene, and benzophenone-3,4,3',4'-tetracarboxylic acid X,X'-diallyl esters Y,Y'-bis(3-(methacryloyloxy)-2-hydroxypropyl)esters. Examples of b) are pentaerythritol tetrathioglycollate, trimethylolpropane trithioglycollate, and 3,6-dioxa-1,8-dimercapto-octane. The compositions may be polymerised by means of actinic irradiation in the presence of an added or "built-in" photo- sensitiser or by the action of a free-radical catalyst. Compositions containing both a photosensitising agent and a heat-activated free- radical catalyst may be subjected to a two-stage process, comprising brief exposure to actinic radiation followed by, when desired, heating. They are useful in the production of surface coatings, adhesive bonds, and of reinforced composites.

367167

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