Adhesive complex coacervates and methods of making and using...

C - Chemistry – Metallurgy – 08 – F

Patent

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C08F 30/02 (2006.01) A61L 24/04 (2006.01) C08J 3/24 (2006.01) C08L 33/00 (2006.01) C08L 43/02 (2006.01) C09J 133/00 (2006.01) C09J 143/02 (2006.01)

Patent

CA 2712843

Described herein is the synthesis of adhesive complex coacervates. The adhesive complex coacervates are composed of a mixture of one or more polycations, one or more poly anions, and one of more multivalent cations. The polycations and polyanions in the adhesice complex coacervate are crosslinked with one another by covalent bonds upon curing. The adhesive complex coacervates have several desirable features when compared to conventional bioadhesives, which are effective in water-based applicatgions. The adhesive complex coacervates described herein exhibit good interfacial tension in water when applied to a substrate (i.e., they spread over the interface rather than being beaded up). Additionally, the ability of the complex coacervate to crosslink intermolecularly increases the cohesive strength of the adhesive complex coacervate. The adhesive complex coacervates have numerous biological applications as bioadhesives and drug delivery devices. In particular, the adhesive complex coacervates described herein are particularly useful in underwater applications and situations where water is present such as, for example, physiological conditions.

La présente invention concerne la synthèse de coacervats adhésifs complexes. Les coacervats adhésifs complexes sont composés d'un mélange d'un ou de plusieurs polycations, d'un ou de plusieurs polyanions et d'un ou de plusieurs cations polyvalents. Les polycations et polyanions présents dans le coacervat adhésif complexe sont réticulés par des liaisons covalentes lors de la polymérisation. Les coacervats adhésifs complexes présentent plusieurs caractéristiques souhaitables comparativement aux bioadhésifs classiques. Ces caractéristiques sont efficaces dans des applications aqueuses. Les coacervats adhésifs complexes décrits dans la présente invention font preuve d'une bonne tension interfaciale dans l'eau lorsqu'ils sont appliqués sur un substrat (c'est-à-dire, bien étalés sur l'interface sans former de bourrelets). De plus, l'aptitude du coacervat complexe à réticuler augmente d'un point de vue intermoléculaire la force cohésive dudit coacervat adhésif complexe. Les coacervats adhésifs complexes ont de nombreuses applications biologiques en tant que bioadhésifs et dispositifs d'administration de médicaments. En particulier, les coacervats adhésifs complexes décrits dans la présente invention se révèlent particulièrement utiles pour des applications subaquatiques et des situations où l'eau est présente telles que, par exemple, les conditions physiologiques.

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