Catalytic production of aryl alkyl hydroperoxides by...

C - Chemistry – Metallurgy – 07 – F

Patent

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C07F 15/02 (2006.01) C07C 37/00 (2006.01) C07C 37/08 (2006.01) C07C 39/04 (2006.01) C07C 45/53 (2006.01) C07C 49/403 (2006.01) C07C 407/00 (2006.01) C07C 409/02 (2006.01) C07C 409/08 (2006.01) C07C 409/10 (2006.01) C07C 409/14 (2006.01) C07F 5/00 (2006.01) C07F 13/00 (2006.01) C07F 15/04 (2006.01) C07F 15/06 (2006.01)

Patent

CA 2250743

A method is provided for preparing organic hydroperoxides by oxidizing aryl alkyl hydrocarbons having a benzylic hydrogen with an oxygen containing gas using as a catalyst an oxo (hydroxo) bridged tetranuclear metal complex having a mixed metal core, one metal of the core being a divalent metal selected from Zn, Cu, Fe, Co, Ni, Mn or mixtures thereof and another metal being a trivalent metal selected from In, Fe, Mn, Ga, and Al. A method is also provided for the manufacture of the catalyst.

Technique de préparation d'hydroperoxydes organiques par oxydation d'arylalkyl-hydrocarbures possédant un hydrogène benzylique avec du gaz contenant de l'oxygène, en employant comme catalyseur un complexe métallique tétranucléaire à pont oxo(hydroxo) ayant un noyau métallique mixte, un métal du noyau étant un métal bivalent choisi parmi Zn, Cu, Fe, Co, Ni, Mn ou des mélanges de ceux-ci, un autre métal étant un métal trivalent choisi parmi In, Fe, Mn, Ga et Al. L'invention porte aussi sur une technique d'obtention du catalyseur.

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