E1 endoglucanase variants y245g, y82r and w42r

C - Chemistry – Metallurgy – 12 – N

Patent

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Details

C12N 9/24 (2006.01) C12N 9/26 (2006.01) C12N 9/42 (2006.01)

Patent

CA 2372594

The invention provides a method for making a glycosyl hydrolase characterized by an increase in catalytic activity on an insoluble substrate, comprising replacing an active site associated glycosyl-stabilizing amino acid of the hydrolase with an amino acid, the replacing amino acid not strongly binding a disaccharide product in the active site, and a method for making a glycosyl hydrolase characterized by an increase in catalytic activity on a soluble substrate, comprising replacing a hydrophobic substrate binding amino acid of the hydrolase with a positively charged amino acid. The invention further provides a glycosyl hydrolase, comprising Y42R (SEQ. ID NO:1), W82R (SEQ. ID NO:2), or Y245G (1) (SEQ. ID NO:3) and the DNA sequences encoding the enzymes.

L'invention concerne un procédé de fabrication d'une glycosyl hydrolase caractérisée par une activité catalytique accrue sur un substrat insoluble. Le procédé consiste à remplacer un acide aminé glycosyl-stabilisant associé au site actif de l'hydrolase par un acide aminé, l'acide aminé de remplacement ne se liant pas fortement à un produit de disaccharide au site actif. L'invention concerne aussi un procédé de fabrication d'une glycosyl hydrolase caractérisée par une activité catalytique accrue sur un substrat soluble, qui consiste à remplacer un acide aminé de l'hydrolase se liant au substrat hydrophobe par un acide aminé chargé positivement. L'invention a en outre trait à une glycosyl hydrolase contenant Y42R (SEQ. ID NO:1), W82R (SEQ. ID NO:2), ou Y245G (1) (SEQ. ID NO:3) et aux séquences d'ADN codant pour ces enzymes.

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