Enzymatic reverse hydrolysis of hydrophilic...

C - Chemistry – Metallurgy – 12 – P

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C12P 21/00 (2006.01) C07K 17/02 (2006.01) C12P 1/00 (2006.01) C12P 7/62 (2006.01) C12P 7/64 (2006.01) C12P 9/00 (2006.01) C12P 13/00 (2006.01) C12P 19/00 (2006.01)

Patent

CA 2101733

The invention relates to methods for he production of amphiphilic pro- ducts such as esters, sugar-esters, pep- tide-esters, glycolipids, glycoproteins, lipoproteins, peptides, and phosphates of alcohols, sugars, and nucleosides. The methods promote enzymatically catalyzed reactions between hydrophil- ic substrates such as glucerol, glucose, amino acids, and nucleosides, and sec- ond substrates such as free fatty acids, triglycerides, vinylesters, amino acids, and phosphates. The method is also applied to enzymatic reactions with saccharides and polyalcohols. The hy- drophilic substrates are adsorbed to finely divided solid supports such as si- lica gel, diatomaceous earths, or acti- vated chracoals in order to promote the dispersion of the hydrophilic substrates within hydrophobic substrates and solvents. Hydrophobic solvents such as n-hexane and t-butylmethylether may be included in the reaction mixtures. Reactions are conducted under non-aqueous conditions in order to promote reverse hydrolysis. Methods are provided for the production of isomerically pure 1,3-diglycerides. Further methods are disclosed for the production and specific precipitation of pure 1- monogycerides through the use of a reactor/separator system. Enzymes used in the methods include lipases from M. mihei and P. fluorescens, glycosidases such as .beta. - galactosidase, proteases such as chymotrypsin, and acid or alkaline phosphatases. Compositions are provided comprising alcohols, carbohydrates, amino acids, or peptides adsorbed onto solid supports such as silica gel.

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