Gas phase process for the epoxidation of non-allylic olefins

C - Chemistry – Metallurgy – 07 – D

Patent

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C07D 303/04 (2006.01) C07D 301/10 (2006.01)

Patent

CA 2173236

Disclosed herein is an improved gas phase process for the selective eposidation of non-allylic olefins wherein the expoxidation is carried out in the presence of certain inert, paraffin hyfrocarbons. Such hydrocarbons possess higher heat capacities as compared to other materials, e.g., nitrogen, argon, methane and helium, typically used as inert diluents in olefin epoxidations. The disclosed process is particularly useful for the continuous manufacture of 3,4-epoxy-1-butene from 1,3-butadiene.

L'invention concerne un procédé en phase gazeuse pour l'époxydation sélective d'oléfines non allyliques dans lequel l'époxydation s'effectue en présence de certains hydrocarbures paraffiniques inertes. Ces hydrocarbures possèdent un pouvoir calorifique supérieur à d'autres corps tels que l'azote, l'argon, le méthane et l'hélium habituellement utilisés en tant que diluants inertes dans l'époxydation d'oléfines. Le procédé selon l'invention est particulièrement utile pour la fabrication en continu de 3,4-époxy-1-butène à partir du 1,3-butadiène.

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