Linear alkylbenzene formation using low temperature ionic...

C - Chemistry – Metallurgy – 07 – C

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C07C 15/107 (2006.01) B01J 31/02 (2006.01) C07C 2/68 (2006.01) C07C 2/86 (2006.01) C07C 211/65 (2006.01) C07F 1/00 (2006.01) C07F 3/00 (2006.01) C07F 5/00 (2006.01) C07F 15/00 (2006.01) H01M 4/36 (2006.01) H01M 6/04 (2006.01) H01M 6/14 (2006.01) H01M 6/16 (2006.01)

Patent

CA 2261735

Linear alkylbenzene compositions can be made by using, as a catalyst, a low temperature molten ionic liquid composition comprising a mixture of a metal halide and a base and, as the alkylating agent for the benzene reagent, a chloroalkane having an average carbon atom content of more than six, an olefin having an average carbon atom content of more than ten, or a mixture of the chloroalkane and the olefin. A novel ionic liquid, which is also useful in other reactions normally catalyzed by previously known ionic liquids, comprises the reaction product of a metal halide, such as aluminum trichloride, and an alkyl-containing amine hydrohalide salt selected from the group consisting of a monoalkyl-, a dialkyl-, a trialkyl-containing amine hydrohalide salt (such as trimethylamine hydrochloride), and mixtures thereof.

On peut préparer des compositions d'alkylbenzène linéaire en utilisant en tant que catalyseur une composition liquide, ionique, fondue et basse température comprenant un mélange d'un halogénure métallique et d'une base, et en tant qu'agent d'alkylation destiné au réactif benzène, un chloroalcane possédant une teneur moyenne en atomes de carbone supérieure à six, une oléfine possédant une teneur moyenne en atomes de carbone supérieure à dix, ou un mélange du chloroalcane et de l'oléfine. Ce nouveau liquide ionique, également utile dans d'autres réactions habituellement catalysées au moyen de liquides ioniques classiques, comprend le produit de réaction d'un halogénure métallique, tel qu'un trichlorure d'aluminium, et un sel d'hydrohalogénure d'amine contenant alkyle, choisi dans le groupe constitué par un sel d'hydrohalogénure d'amine contenant monoalkyle, dialkyle ou trialkyle (tel qu'un hydrochlorure de triméthylamine).

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