Method for characterizing polypeptides

G - Physics – 01 – N

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G01N 33/68 (2006.01) C07K 1/12 (2006.01)

Patent

CA 2449680

Provided is a method for characterising a polypeptide, which method comprises the steps of: (a) optionnally reducing cysteine disulphide bridges in the polypeptide to form free thiols, and capping the free thiols; (b) cleaving the polypeptide with a sequence specific cleavage reagent to form peptide fragments; (c) optionally deactivating the cleavage reagent; (d) capping one or more .epsilon.-amino groups that are present with a lysine reactive agent; (e) analysing peptide fragments by mass spectrometry to form a mass fingerprint for the polypeptide; and (f) determining the identity of the polypeptide from the mass fingerprint.

Le procédé de caractérisation de polypeptides de la présente invention enchaîne les opérations suivantes. (a) Réduction éventuelle des ponts de bisulfure de cystéine du polypeptide pour donner des thiols libres et coiffage des thiols libres. (b) Clivage du polypeptide avec un réactant de clivage spécifique de la séquence pour donner des fragments de peptides. (c) Désactivation éventuelle du réactant de clivage. (d) Coiffage de l'un au moins des groupes .epsilon.-aminés présents avec un agent réagissant à la lysine. (e) Analyse des fragments du peptide par spectrométrie de masse pour former une empreinte de masse pour le polypeptide. Enfin (f), détermination de l'identité du polypeptide à partir de l'empreinte de masse.

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