Method for fluorinating a compound comprising a...

C - Chemistry – Metallurgy – 01 – B

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C01B 21/092 (2006.01) C01B 21/093 (2006.01) C01B 21/097 (2006.01) C07C 303/02 (2006.01) C07C 303/36 (2006.01) C07C 311/48 (2006.01) H01M 10/40 (2006.01)

Patent

CA 2432053

The invention concerns a fluorination method for obtaining fluorinated compounds. The method consists in reacting with an ionic fluoride of a monovalent cation a compound of formula (I), wherein: M represents H, an alkaline metal, a quaternary phosphonium group or a quaternary ammonium group; Y represents SO¿2?, and m is 1, or Y is PO and m is 2; Z represents CR?2¿, N or P; R?1¿ represents a carbonaceous and/or electron-attracting group which has a Hammet parameter .sigma.¿P? higher than 0.4; R?2¿ represents a carbonaceous and/or electron-attracting group; X represents a halogen other than a fluorine. The fluorinated compounds obtained are useful in particular as electrolyte in lithium batteries.

L'invention concerne un procédé de fluoration pour l'obtention de composés fluorés.Le procédé consiste à faire réagir un composé (I) répondant à la formule voir formule avec un fluorure ionique d'un cation monovalent. M représente H, un métal alcalin, un groupe phosphonium quaternaire ou un groupe ammonium quaternaire. Y représente SO2 et m est 1, ou bien Y est PO et m est 2. Z représente CR2, N ou P. R1 représente un groupe électro-attracteur qui a un paramètre sP de Hammet supérieur à 0,4. R2 représente un groupe carboné et/ou électro-attracteur. X représente un halogène différent d'un fluor.Les composés fluorés obtenus sont utiles notamment comme électrolyte dans les batteries au lithium.

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