Method for producing alcoxylated carbonyl compounds by an...

C - Chemistry – Metallurgy – 25 – B

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C25B 3/02 (2006.01) C07C 41/50 (2006.01) C07C 41/60 (2006.01)

Patent

CA 2429450

A method for producing alcoxylated carbonyl compounds of general formula (I) (compounds I): R1aR2C(OR3)b wherein R1, R2 represent hydrogen or C1- C6-alkyl, R3 independently means C1- C6-alkyl, a is 0 or 1, b 2 or 3 with the proviso that the sum of a and b is 3, by means of anodic oxidation of germinal dialcoxy compounds of general formula (II) (compounds II) wherein R4, R5, R6, R7 represent hydrogen or C1- C6-alkyl, R5, R6 represent C1- C6-alkyl or C1- C6- alcoxy, in the presence of a C1-C6-alkyl alcohol (compounds III).A usual compound (compound IV) is used as a cathodic depolarizer suitable for electrochemical oxidation. The anodic oxidation and cathodic reduction is carried out in an undivided electrolyte cell in the presence of C1-C6-alkyl alcohols.

L'invention concerne un procédé pour produire des liaisons carbonyle alcoxylées de formule générale (I) (liaisons I): R?1¿¿a?R?2¿C(OR?3¿)¿b? dans laquelle R?1¿, R?2¿ signifient hydrogène ou alkyle C¿1? à C¿6?, R?3¿ représente indépendamment alkyle C¿1? à C¿6?, a est 0 ou 1, b est 2 ou 3, sous réserve que la somme de a et b est égale à 3. Le procédé comprend l'oxydation anodique de liaisons dialcoxy géminales de formule générale (II) (liaisons II), dans laquelle R?4¿, R?5¿, R?6¿, R?7¿ signifient hydrogène ou alkyle C¿1? à C¿6?, R?5¿, R?6¿ représentent alkyle C¿1? à C¿6? ou alcoxy C¿1? à C¿6? en présence d'un alcool alkyle C¿1? à C¿6? (liaisons III). On utilise comme dépolarisateur cathodique une liaison organique classique (liaison IV) adaptée à l'oxydation électrochimique. L'oxydation anodique et la réduction cathodique sont réalisées dans une cellule électrolytique non divisée en présence d'alcools alkyle C¿1?-C¿6?.

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