Method to control increase in viscosity during aging of...

C - Chemistry – Metallurgy – 08 – L

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C08L 9/06 (2006.01) C08J 3/20 (2006.01) C08K 5/5419 (2006.01) C08L 101/02 (2006.01)

Patent

CA 2380082

A method for controlling any increase in Mooney viscosity during aging of siloxane-functionalized polymers in-cludes the step of adding a viscosity stabilizing effective amount of a viscosity stabilizing agent selected from the group consisting of alkyl alkoxysilanes of the structural formula R1n Si(OR2)4-n wherein R1 is selected from the group consisting of C1 to C20 alkyl, C4 to C10 cycloalkyl, or C5 to C20 aromatic groups, wherein R2 may be the same as or different from R1 and is selected from the group consisting of C1 to C20 alkyl, C4 to C10 cycloalkyl, or C5 to C20 aromatic groups, and wherein n is an integer from 1 to 3. The method provides for the stabilization of Mooney viscosity of siloxane-functionalized polymers at any given level upon aging. The viscosity stabilizing agents react with the siloxane-functionalized polymers during hydrolysis of the siloxane end groups to form moisture stabilized polymers.

L'invention concerne un procédé de régulation de toute augmentation de la viscosité de Mooney pendant le vieillissement de polymères à fonctionnalité siloxane. Ledit procédé consiste à ajouter une dose efficace stabilisant la viscosité, d'un agent de stabilisation de viscosité choisi dans le groupe formé d'alcoxysilanes alkyliques de formule structurale R<1>nSi(OR<2>)4-n, R<1> étant choisi dans le groupe formé d'alkyle C1-C20, de cycloalkyle C4 à C10, ou de groupes aromatiques C5 à C20, R<2> pouvant être identique ou différent de R<1> et choisi dans le groupe constitué d'alkyle C1 à C20, de cycloalkyle C4 à C10, ou de groupes aromatiques C5 à C20, et n valant un entier de 1 à 3. Ledit procédé permet la stabilisation de la viscosité de Mooney de polymères à fonctionnalité siloxane à n'importe quel stade du vieillissement. Les agents de stabilisation de la viscosité réagissent avec les polymères à fonctionnalité siloxane, pendant l'hydrolyse des groupes d'extrémité siloxanes, de sorte que des polymères stabilisés à l'humidité soient formés.

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