Preparation of mono epoxides and tertiary butyl alcohol...

C - Chemistry – Metallurgy – 07 – C

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C07C 31/12 (2006.01) B01J 31/40 (2006.01) C07C 29/132 (2006.01) C07D 301/19 (2006.01) C07D 301/32 (2006.01) C07D 303/04 (2006.01)

Patent

CA 2087237

PREPARATION OF MONO EPOXIDES AND TERTIARY BUTYL ALCOHOL USING REGENERATED CATALYST (Docket No. 81,021-F) ABSTRACT OF THE DISCLOSURE In the preparation of tertiary butyl alcohol and a linear C3-C12 mono epoxide by the epoxidation reaction of a linear C3- C12 alpha mono olefin with tertiary butyl hydroperoxide in solution in tertiary butyl alcohol in the presence of a catalytic amount of a soluble complex of molybdenum with ethylene glycol, a portion of the catalyst that is used is a recycle (final) ethylene glycol solution of a complex of ethylene glycol with ammonium-containing molybdenum compounds prepared from ethylene glycol and a precipitate of solid ammonium-containing molybdenum compounds formed by saturating a heavy distillation fraction with ammonia to thereby form a liquid amination product containing a precipitate of solid ammonium-containing molybdenum compounds; the heavy distilla- tion fraction being obtained by distillation of the epoxida- tion reaction product.

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