Preparation of taxol and docetaxel through primary amines

C - Chemistry – Metallurgy – 07 – D

Patent

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C07D 305/14 (2006.01) C07F 7/10 (2006.01) C07H 15/26 (2006.01)

Patent

CA 2211799

The invention relates to a process for converting Taxol A, B and C to Taxol primary amine which can then be easily and efficiently converted to Taxol A or docetaxel, thereby significantly increasing the yield of these products from biomass. The method includes the removal of the amide from the side-chain with Schwartz's reagent to form an imine, followed by the hydrolysis of the imine to the primary amine. The primary amine can then be converted to Taxol A or docetaxel. New Taxol imine compounds and primary amine salts have been formed by this process.

La présente invention concerne un procédé de conversion de Taxol A, B et C en amine primaire du Taxol qui peut être ensuite facilement et efficacement convertie en Taxol A ou docetaxel, accroissant par là de façon importante la production de ces produits issus de la biomasse. Le procédé consiste notamment à retirer l'amide de la chaîne latérale au moyen du réactif de Schwartz afin de former une imine, puis à hydrolyser l'imine en amine primaire. Cette amine primaire peut ensuite être convertie en Taxol A ou en docetaxel. Les composés imine du Taxol et les sels d'amines primaires de la présente invention ont été formés selon ce procédé.

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