Process for carbonylation of aliphatic alcohols and/or...

C - Chemistry – Metallurgy – 07 – C

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C07C 67/37 (2006.01) C07C 51/12 (2006.01) C07C 53/08 (2006.01) C07C 69/14 (2006.01)

Patent

CA 2671361

A product comprising a C1-C3 aliphatic carbbxylic acid or corresponding ester is produced by a process comprising reacting a C1-C3 aliphatic alcohol or a reactive derivative thereof with carbon monoxide in the presence of a zeolite catalyst having an 8-member ring channel which is interconnected with a channel defined by a ring with greater than or equal to 8 members, the 8-member ring having a window size of at least 2.5 Angstroms x at least 3.6 Angstroms and at least one Brønsted acid site and the zeolite having a silica : X2O3 ratio of at least 5, wherein X is selected from aluminium, boron, iron, gallium and mixtures thereof with the proviso that the zeolite is not mordenite or ferrierite.

Un produit comprenant un acide carboxylique aliphatique en C1 à C3 ou un ester correspondant est produit par un procédé comprenant la réaction d'un alcool aliphatique en C1 à C3 ou de l'un de ses dérivés réactifs avec du monoxyde de carbone en présence d'un catalyseur de zéolite présentant un canal cyclique à 8 chaînons qui est interconnecté avec un canal défini par un cycle à 8 chaînons ou plus, le cycle à 8 chaînons présentant une taille de fenêtre d'au moins 2,5 Angströms x, au moins 3,6 Angströms et au moins un site d'acide de Bronsted et la zéolite présentant un rapport de silice / X2O3 d'au moins 5, X étant choisi parmi l'aluminium, le bore, le fer, le gallium et leurs mélanges à condition que la zéolite ne soit pas de la mordénite ou de la ferriérite.

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