Process for converting methanol to alkyl ethers, gasol ine...

C - Chemistry – Metallurgy – 07 – C

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260/648, 260/707

C07C 2/62 (2006.01) C07C 1/20 (2006.01) C07C 9/16 (2006.01) C07C 41/06 (2006.01) C07C 43/04 (2006.01) C10G 3/00 (2006.01) C10G 29/20 (2006.01) C10L 1/02 (2006.01) C10L 1/18 (2006.01)

Patent

CA 1275420

IMPROVED PROCESS FOR CONVERTING METHANOL TO ALKYL ETHERS ABSTRACT A multistage process for producing isoalkyl ethers from lower aliphatic oxygenate feedstock, such as methanol. Feedstock is catalytically converted in a primary catalyst stage at elevated temperature in contact with zeolite catalyst to predominantly C2-C7 lower olefins comprising isobutylene and isoamylene, by-product water and a minor amount of C8+ hydrocarbons, followed by fractionation of the C2-C7 olefins to recover a C2-C3-rich recycle stream for further catalytic conversion in the primary stage. C4-C7 olefins are passed to a second catalytic etherification stage for reaction of isoalkenes with methanol to produce methyl tertiary-butyl ether, methyl isoamylether and higher isoalkyl ethers. The second stage effluent may be fractionated to recover an ether product, C5+ hydrocarbon liquid product, and unreacted butenes. Advantageously, the unreacted butenes are further reacted with isoparaffin in a third catalytic stage under acid catalysis alkylation conditions, and fractionated to recover C6+ alkylate liquid, liquid hydrocarbon product. The ethers may be blended with at least one C6+ hydrocarbon to produce high octane gasoline.

542219

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