Process for decreasing chlorine content in chlorinated...

C - Chemistry – Metallurgy – 07 – C

Patent

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Details

C07C 25/00 (2006.01) C07B 35/06 (2006.01) C07C 17/23 (2006.01) A62D 3/00 (2006.01)

Patent

CA 2173970

The chlorine or halide content in a chlorinated hydrocarbon or halogenated aromatic hydrocarbon in an environment which admits to the presence of air and moisture can be reduced by bringing the chlorinated hydrocarbon or halogenated aromatic hydrocarbon into contact with a reagent which comprises (i) a complex of a substantially nontoxic metal having at least two oxidation states and (ii) a reducing agent which reductively returns the complex from its second oxidation step to its first oxidation stage. A representative embodiment involves bis-(5-cyclopentadienyl)titanium dichloride and sodium tetrahydridoborate. Optionally, the reaction is conducted in the presence of an aliphatic or aromatic amine, optionally in the presence of an inert organic solvent.

On peut réduire la teneur en chlore ou en halogénure dans un hydrocarbure chloré ou dans un hydrocarbure aromatique halogéné, dans un environnement qui admet la présence de l'air et de l'humidité, en mettant en contact l'hydrocarbure chloré ou l'hydrocarbure aromatique halogéné avec un réactif qui comprend: (i) un complexe d'un métal sensiblement non toxique possédant au moins deux états d'oxydation, et (ii) un agent de réduction qui réduit le complexe en le renvoyant de son second état d'oxydation à son premier état d'oxydation. Un mode de réalisation représentatif de cette invention utilise le bis-(??5¿-cyclopentadiényl) dichlorure de titane et le tétrahydridoborate de sodium. Eventuellement, la réaction peut être conduite en présence d'une amine aliphatique ou aromatique, éventuellement en présence d'un solvant organique inerte.

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