Process for obtaining quinapryl hydrochloride and solvates...

C - Chemistry – Metallurgy – 07 – D

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C07D 217/26 (2006.01)

Patent

CA 2293705

The process for obtaining quinapril hydrochloride (I) comprises the stages of: a) hydrogenolysis of the benzyl ester of quinapril (II) by treatment in an alcoholic solvent, with concentrated hydrochloric acid or a solution of hydrogen chloride in isopropanol, and hydrogenation; b) removal of the solvent; c) addition of toluene to precipitate the quinapril hydrochloride as a toluene solvate; d) treatment of said solvate with a Class 3 solvent which forms a solvate of quinapril hydrochloride from which it can be removed by drying without degrading; and e) drying of the solvate from step d) to yield quinapril hydrochloride (I), an antihypertensive agent.

L'invention concerne un procédé permettant d'obtenir du chlorhydrate de quinapryl (I) consistant à a) effectuer une hydrogénolyse de l'ester benzylique du quinapryl (II) par traitement dans un solvant alcoolique, avec acide chlorhydrique ou avec un chlorure d'hydrogène dissous dans l'isopropanol, et par hydrogénation; à b) retirer le solvant; à c) ajouter du toluène pour précipiter le quinapryl chlorhydrate comme solvate de toluène; à d) traiter ledit solvate avec un solvant de la classe 3 qui forme un solvate de chlorhydrate de quinapryl à partir duquel on peut l'éliminer par séchage sans le dégrader; et à e) sécher le solvate de l'étape d) pour obtenir (I). Ces solvates sont utiles pour isoler et purifier (I) un agent antihypertenseur.

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