Process for the preparation of macrocyclic compounds by...

C - Chemistry – Metallurgy – 07 – K

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C07K 5/08 (2006.01) B01J 31/22 (2006.01) C07C 6/06 (2006.01) C07F 15/00 (2006.01) C07K 1/08 (2006.01) C07K 1/113 (2006.01) C07K 5/06 (2006.01)

Patent

CA 2521835

The invention relates to an improved process for the preparation of a macrocyclic compound of formula I wherein R1, R2, R3, A and D have the meaning given in the claims; by a ring closure metathesis of the corresponding diene of formula III wherein R1, R2, R3, A and D' have the meaning given in the claims; in the presence of a benzylidene ruthenium catalyst, wherein the phenyl group is substituted by a nitro group.

La présente invention concerne un procédé amélioré pour préparer un composé macrocyclique de formule (I), dans laquelle R¿1?, R?2¿, R?3¿, A et D ont la signification donnée dans les revendications, par métathèse à cyclisation du diène correspondant de formule (III), dans laquelle R¿1?, R?2¿, R?3¿, A et D' ont la signification donnée dans les revendications, en présence d'un catalyseur de ruthénium benzylidène, le groupe phényle étant substitué par un groupe nitro.

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