Process for the preparation of the methyl ester of...

C - Chemistry – Metallurgy – 07 – C

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260/488

C07C 69/716 (2006.01)

Patent

CA 1148563

PROCESS FOR THE PREPARATION OF THE METHYL ESTER OF 4-OXOPENTANE-1-CARBOXYLIC ACID ABSTRACT OF THE DISCLOSURE An improved process for the preparation of the methyl ester of 4-oxopentane-1-carboxylic acid by the reaction of acetone with methyl acrylate. The reactants are reacted in a reaction zone in the presence of both a primary amine and/or Schiff base as a catalyst, and an acid compound to form a reaction mixture containing the methyl ester. The reaction mixture is distilled to form a distillate containing unconsumed reactants and catalyst and a residual liquid phase containing the methyl ester. The distillate is recycled to the reaction zone, and the methyl ester is recovered from the residual liquid phase by a further distillation. The amount of oxygen dissolved in the reaction mixture is maintained at a level below 20 parts by weight per million, and the distillation of the reaction mixture is carried out at a temperature of less than 195°C, at a pressure of at least atmospheric, and in the presence of an inert solvent having a boiling point of between 80 and 195°C.

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