Process for the production of ge by reduction of geci4, with...

C - Chemistry – Metallurgy – 22 – B

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C22B 41/00 (2006.01) C22B 5/04 (2006.01)

Patent

CA 2580398

The invention relates to the manufacture of high purity germanium for the manufacture of e.g. infra red optics, radiation detectors and electronic devices. GeCl4 is converted to Ge metal by contacting gaseous GeCl4 with a liquid metal M containing one of Zn, Na and Mg, thereby obtaining a Ge-bearing alloy and a metal M chloride, which is removed by evaporation or skimming. The Ge-bearing alloy is then purified at a temperature above the boiling point of metal M. This process does not require complicated technologies and preserves the high purity of the GeCl4 in the final Ge metal, as the only reactant is metal M, which can be obtained in very high purity grades and continuously recycled.

L'invention concerne la fabrication de germanium de pureté élevée destiné à la fabrication, par exemple, d'éléments optiques infrarouge, de détecteurs de rayonnements et de dispositifs électroniques. GeCl4 est converti en métal Ge par mise en contact de GeCl4 gazeux avec du métal liquide M renfermant un élément parmi Zn, Na et Mg, de manière à obtenir un alliage renfermant du Ge et un chlorure de métal M, éliminé par évaporation ou écrémage. L'alliage renfermant du Ge est ensuite purifié à une température supérieure au point d'ébullition du métal M. Ce procédé ne nécessite pas de technologies complexes et conserve la pureté élevée du GeCl4 dans le métal Ge final, du fait que le seul réactif est le métal M, pouvant être obtenu à des degrés de pureté très élevés et être recyclé en continu.

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