Selective, catalytic, thermal functionalization of secondary...

Details Selective, catalytic, thermal functionalization of secondary... Selective, catalytic, thermal functionalization of secondary...

C - Chemistry, Metallurgy

07

B

C07B 47/00 (2006.01) C07F 5/02 (2006.01)

Patent

CA 2480571

A catalytic process having more than 50 turnovers comprises thermally activating a catalysis, in the presence of a functionalizing reagent and a cyclic hydrocarbon comprising an aromatic compound or a cycloparaffin compound lacking primary C-H bonds. The catalyst comprises (a) a source of a transition metal; (b) a source of a 3 to 8, cyclic or non-cyclic, aromatic or non-aromatic, neutral, cationic or anionic, substituted or unsubstituted, electron donor moiety which does not dissociate under thermal reaction conditions; a.nd (c) a source of ligands capable of formally donating an electron pair to the transition metal (a) and which dissociate thermally; and wherein said functionalizing reagent comprises a source of B, C, N, O, Si, P, S, Ge, As, Al, or Se.

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