Synthesis of energetic polyester thermoplastic homopolymers...

C - Chemistry – Metallurgy – 08 – G

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C08G 63/08 (2006.01) C06B 45/10 (2006.01) C08G 63/685 (2006.01) C08G 63/91 (2006.01)

Patent

CA 2367795

Polymerization of .alpha.-bromomethyl-.alpha.-methyl-.beta.-propiolactone (BMMPL) or .alpha.- chloromethyl-.alpha.-methyl-.beta.-propiolactone (CMMPL) yielded thermoplastic homopolymers that upon azidation led to a novel energetic thermoplastic polyester: poly(.alpha.-azidomethyl-.alpha.- methyl-.beta.-propiolactone) (PAMMPL). An energetic copolyether-ester thermoplastic elastomer was prepared by using glycidyl azide polymer, a dihydroxyl terminated energetic polymer, as a macroinitiator for the polymerization of BMMPL or CMMPL. The azidation of the resulting copolyether-ester yielded an energetic thermoplastic elastomer that melted at between 80°C and 85°C. Polymerization of .alpha.-dibromomethyl- .beta.-propiolactone (DBMPL) resulted in a polymer which upon azidation yielded a new energetic polymer that can be used as a binder or into an energetic thermoplastic elastomer synthesis.

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