Process for purifying and recovering catalyst solution...

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B01J 38/52 (2006.01) B01J 31/40 (2006.01) C07C 43/04 (2006.01) C07C 69/14 (2006.01)

Patent

CA 1280400

PROCESS FOR PURIFYING AND RECOVERING CATALYST SOLUTION CONTAMINATED DURING THE CARBONYLATION OF METHYL ACETATE AND/OR DIMETHYLETHER ABSTRACT OF THE DISCLOSURE Catalyst solution contaminated during the carbonyla- tion of methyl acetate and/or dimethylether. To this end, the contaminated catalyst solution is subjected in a first processing stage to extraction with a dialkylether and al- kanol, each of which has from 1-4 carbon atoms per alkyl group, and thereby freed from its organic contaminants, from acetic acid, acetic anhydride and ethylidene diace- tate, and the ether phase is separated from the purified promoter-containing catalyst solution; next, the ether phase is treated in a second processing stage with iodine and/or methyl iodide; the precipitated promotercontaining catalyst complex is separated and dissolved in the puri- fied catalyst solution coming from the first processing stage; the ether phase is separated into its constituents by distilling it; recovered dialkylether and alkanol are used again in the extraction stage; fresh catalyst solu- tion is prepared from the recovered mixture of acetic acid, acetic anhydride and ethylidene diacetate and from the united purified catalyst solution while residual di- alkylether and alkanol are distilled off, and the organic contaminants retained in the residue of the ether phase distillation are expelled.

533015

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