Polymer electrolytes crosslinked by ultraviolet radiation

C - Chemistry – Metallurgy – 08 – J

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C08J 3/28 (2006.01) C08F 214/18 (2006.01) C08F 214/26 (2006.01)

Patent

CA 2549085

A method is provided for making a crosslinked polymer electrolyte, typically in the form of a membrane for use as a polymer electrolyte membrane in an electrolytic cell such as a fuel cell, as well as the polymer so made, the method comprising application of ultraviolet radiation to a highly fluorinated fluoropolymer comprising: a backbone derived in part from tetrafluoro-ethylene monomer, first pendent groups which include a group according to the formula - SO2X, where X is F, Cl, Br, OH or -O-M+, where M+ is a monovalent cation, and second pendent groups which include Br, Cl or I. Typically, the membrane has a thickness of 90 microns or less, more typically 60 or less, and most typically 30 microns or less.

L'invention concerne une méthode pour fabriquer un électrolyte polymère réticulé; typiquement sous la forme d'une membrane à utiliser en tant que membrane d'électrolyte primaire dans une cellule électrolytique, notamment une pile à combustible, ainsi que le polymère ainsi fabriqué. La méthode de l'invention consiste à appliquer un rayonnement ultraviolet sur un fluoropolymère hautement fluoré comprenant: un squelette dérivé en partie à partir d'un monomère de tétrafluoro-éthylène, des premiers groupes latéraux comprenant un groupe de formule -SO¿2?X, dans laquelle X désigne F, Cl, Br, OH ou -O?-¿M?+¿, M désignant un cation monovalent, et des seconds groupes latéraux comprenant Br, Cl ou I. Typiquement, la membrane présente une épaisseur inférieure ou égale à 90 microns, de préférence, typiquement inférieure à 60 microns, et idéalement, typiquement inférieure ou égale à 30 microns. ? ¿

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