Process for polymerizing cyclical olefins and...

C - Chemistry – Metallurgy – 08 – G

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C08G 61/08 (2006.01) G03F 7/031 (2006.01)

Patent

CA 2205458

The invention concerns a process for the photocatalytic polymerization of a cyclical olefin or of at least two different cyclical olefins in the presence of a metal compound as catalyst. Photochemical ring-opening metathesis polymerization is carried out in the presence of a catalytic amount of at least one heat-stable titanium(IV), niobium(V), tantalum(V), molybdenum(VI) or tungsten(VI) compound in which a silylmethyl group and at least one halogen are bonded to the metal. The process can also be carried out such that irradiation is firstly performed, followed by polymerization by heating. The process is used, for example, for producing thermoplastics shaping compounds, coatings and images in relief.

L'invention concerne un procédé de polymérisation photocatalytique d'une oléfine cyclique ou d'au moins deux oléfines cycliques différentes en présence d'un composé métal servant de catalyseur. On effectue une polymérisation par métathèse avec ouverture du cycle en présence d'un volume catalytique d'au moins un composé titane(IV), niobium(V), tantale(V), molybdène(VI) ou tungstène(VI) thermostable, où un groupe méthyle de silyle et au moins un halogène sont liés au métal. On peut également appliquer ce procédé en commençant par l'irradiation, et en terminant par la polymérisation par chauffage. Ce procédé s'utilise par exemple pour produire des matières moulées, des revêtements et des représentations en relief thermoplastiques.

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