Process for the production of dinitrotoluene and isomeric...

C - Chemistry – Metallurgy – 07 – C

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C07C 205/06 (2006.01) C07C 201/08 (2006.01)

Patent

CA 2178699

Dinitrotoluene and isomer mixtures of dinitrotoluene are produced in a single stage, continuous process by nitrating mononitrotuluene or an isomer mixture of mononitrotoluene in which the ortho-mononitrotoluene content is low with a nitrating acid made up of (1) from about 80 to about 100 wt.% inorganic constituents and (2) up to 20 wt.% organic constituents. The inorganic constituents of the nitrating acid include: (a) from about 60 to about 90 wt.% sulfuric acid, (b) from about 1 to about 20 wt.% nitric acid, and (c) at least 5 wt.% water. The organic constituents of the nitrating acid include: from about 70 to about 100 % by weight nitrotoluene isomers and up to about 30% by weight nitration by-products. The nitration reaction is carried out under adiabatic conditions. The molar ratio of nitric acid to mononitrotoluene during the nitration reaction is generally from about 0.7:1 to about 1.4:1. The phases generated during the nitration are subsequently separated and the acid phase is treated to remove at least 5 wt.% of the water present therein. The water may be removed by distillation or flash vaporization, optionally with simultaneous heat supply. After removal of the water, nitric acid having a concentration of from about 50 to about 100 wt.% is added to the treated acid phase in amount sufficient to satisfy the compositional limits for a nitrating acid useful in the process of the present invention. This reconcentrated acid phase is then returned to the nitration reaction.

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