Antireflective graded index silica coating, method for...

C - Chemistry – Metallurgy – 03 – C

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117/101, 6/226

C03C 17/02 (2006.01) C03C 15/00 (2006.01) C03C 17/27 (2006.01) G02B 1/10 (2006.01) G02B 1/11 (2006.01)

Patent

CA 1218507

51,141 ABSTRACT OF THE DISCLOSURE Antireflective silica coating for vitreous material is substantially non-reflecting over a wide band of radiations. This is achieved by providing the coating with a graded degree of porosity which grades the index of refraction between that of air and the vitreous material of the substrate. To prepare the coating, there is first prepared a silicon-alkoxide-based coating solution of particular polymer structure produced by a controlled proportion of water to alkoxide and a controlled concen- tration of alkoxide to solution, along with a small amount of catalyst. The primary solvent is alcohol and the solution is polymerized and hyrolized under controlled conditions prior to use. The prepared solution is applied as a film to the vitreous substrate and rapidly dried. It is thereafter heated under controlled conditions to vola- tilize the hydroxyl radicals and organics therefrom and then to produce a suitable pore morphology in the residual porous silica layer. The silica layer is then etched in order to enlarge the pores in a graded fashion, with the largest of the pores remaining being sufficiently small that radiations to be passed through the substrate are not significantly scattered. For use with quartz substrates, extremely durable coatings which display only 0.1% reflec- tivity have been prepared.

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