Preparation of methacrylic acid

C - Chemistry – Metallurgy – 07 – C

Patent

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260/520.7

C07C 51/235 (2006.01) C07C 51/25 (2006.01) C07C 57/05 (2006.01)

Patent

CA 1309418

Abstract of the Disclosure: Methacrylic acid can be pre- pared with advantage by gas phase oxidation of methacrolein or isobutyraldehyde over Mo- and P-containing catalysts at from 250 to 400°C with cooling of the hot reaction gas to below 100°C, absorption of the methacrylic acid in a water- operated absorption column, at below 100°C and partial re- cycling into the oxidation reactor after admixture of meth- acrolein or isobutyraldehyde and oxygen by feeding a quan- tity of methacrolein or isobutyraldehyde equal to the quan- tity of methacrolein or isobutyraldehyde consumed in the reaction in liquid form together with a polymerization inhibitor into the reactor gas in the lower two-thirds of the absorption column and upstream of the feed point for the fresh methacrolein or isobutyraldehyde or down-stream of the absorption column splitting off the reactor off-gas. a side stream which is washed in a wash column operated with water at < 10°C to remove unconverted methacrolein or isobutyraldehyde which is fed as an aqueous solution to the top of the absorption column.

570525

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